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Just yesterday, I harvested wild grapes, cut some grave vine wood, from a dead vine, for a new wand(Correspondence=Joy).
I also harvested a nice pile of wild mistletoe(all heal-Sacred herb of the Druids; one of the three ingredients in Medieval True Love Powder.)
Guerilla Gardening is SIMPLE; go outside and walk along on non-private property until you find something that you want to harvest. Then make a decision.... take it all, or take some and tend to the growth of what you leave.
Try this; set a goal of finding just one plant that you like, weather you recognize it or not doesn't matter. When you find it take some pics, and mark it on a map(I use google maps). Go home a research it. If its a keeper, go back and receive it as a gift from mother father god.
If you do this three times and you dont become EXTREMELY addicted..... just revert to ordering herbs off the internet, and focus on something besides gardening.
Ill post some grape and mistletoe pics in a min.